To create the brush is used a large amount of simple brush dots in various sizes, shades and with varying edge softnesses. I then used the chalk brush around the edges in order to break up the outline of the cloud shape in order to make it look slightly softer. I also used a little bit of the smudge tool as this was an extremely effective way of adding a little bit of a swirl to it.
Below are the custom brush I made and the simple sky image that I created using the brush.
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